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1 article(s) from Stefano, Luciano H. Di

Tailoring of organic dyes with oxidoreductive compounds to obtain photocyclic radical generator systems exhibiting photocatalytic behavior

Christian Ley,
Julien Christmann,
Ahmad Ibrahim,
Luciano H. Di Stefano and
Xavier Allonas

Beilstein J. Org. Chem. 2014, 10, 936–947, doi:10.3762/bjoc.10.92

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Graphical Abstract

Scheme 1: Chemical structures of RB, EDB and TA.

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Scheme 2: Type II PIS mechanisms. PS: photosensitizer; ^1,3PS^*: singlet and triplet PS excited states; PS^•+: o...

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Figure 1: Evolution of RB concentration as a function of irradiation time (λ = 532 nm, 9 mW·cm⁻³); insert: ab...

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Scheme 3: Photocatalytic behavior occurring in three component PIS. PS: photosensitizer; ^1,3PS^*: singlet and ...

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Figure 2: Evolution of [RB](t) in the photocyclic system RB/TA/EDB as a function of irradiation time (λ = 532...

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Scheme 4: Thermodynamics of an oxidative three components PCIS, a) ground state reaction ( [Graphic 1] ), b) excited state...

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Scheme 5: General photocatalytic cycle occurring in three components photocyclic systems. Two cycles are in c...

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Figure 3: Mechanistic description of photocyclic system involved in the RB/TA/EDB system. The rate constants ...

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Figure 4: Evolution of RB, RB^•+, TA, and TA^•− concentration with time for RB/TA system.

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Figure 5: Evolution of RB, TA and EDB concentrations in the photocyclic system. The logarithm of oxidative an...

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Figure 6: Evolution of radical concentrations TA^•− and EDB^•+ together with [RB] in photocatalytic system.

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Full Research Paper

Published 25 Apr 2014

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